Ni-W-GO-Al2O3复合镀层的制备及其耐磨耐蚀性能Preparation of Ni-W-GO-Al2O3 composite coatings and its wear and corrosion resistance
田水昌,崔洪芝,张国松,王欢欢
摘要(Abstract):
首先采用纳米Al_2O_3颗粒对氧化石墨烯(GO)进行表面改性,然后利用脉冲电沉积技术在碳钢表面制备了Ni-W-GO-Al_2O_3复合镀层,采用扫描电镜、摩擦磨损试验机和电化学工作站等研究了复合镀层的形貌、组织结构及耐磨耐蚀性能。结果表明:Al_2O_3的加入抑制了GO团聚,有助于镀层组织均匀化;与单纯的Ni-W-GO镀层相比,Ni-W-GO-0.3Al_2O_3镀层表面平整、致密无裂纹,耐磨耐蚀性能最好;Al_2O_3添加量过低,起不到抑制GO团聚的效果;添加量过高,Al_2O_3发生自发团聚,形成大量裂纹,既降低镀层的耐蚀性,同时也降低耐磨性。
关键词(KeyWords): Ni-W-GO-Al_2O_3;电沉积;复合镀层;耐磨性;耐腐蚀性
基金项目(Foundation): 国家高技术研究发展计划(863计划)(2015AA034404);; 国家自然科学基金(51772176);; 泰山学者攀登计划(tspd20161006)
作者(Author): 田水昌,崔洪芝,张国松,王欢欢
DOI: 10.13289/j.issn.1009-6264.2018-0450
参考文献(References):
- [1] Lee H B.Synergy between corrosion and wear of electrodeposited Ni-W coating[J].Tribology Letters,2013,50(3):407-419.
- [2] Yari S,Dehghanian C.Deposition and characterization of nanocrystalline and amorphous Ni-W coatings with embedded alumina nanoparticles[J].Ceramics International,2013,39(7):7759-7766.
- [3] Aliofkhazraei M,Ahangarani S,Rouhaghdam A S.Effect of the duty cycle of pulsed current on nanocomposite layers formed by pulsed electrodeposition[J].Rare Metals,2010,29(2):209-213.
- [4] Gyawali G,Joshi B,Tripathi K,et al.Preparation of Ni-W-Si3N4,composite coatings and evaluation of their scratch resistance properties[J].Ceramics International,2016,42(2):3497-3503.
- [5] Huang Y,Huang F,Zhao W,et al.The study of electroless Ni-W-P alloy plating on glass fibers[J].Rare Metals,2007,26(4):365-371.
- [6] Beltowska-Lehman E,Indyka P,Bigos A,et al.Ni-W/ZrO2,nanocomposites obtained by ultrasonic DC electrodeposition[J].Materials and Design,2015,80(5):1-11.
- [7] Hosseini M G,Abdolmaleki M,Ghahremani J.Investigation of corrosion resistance of electrodeposited Ni-W/SiC composite coatings[J].Corrosion Engineering Science and Technology,2014,49(4):247-253.
- [8] Ma C,Liang G,Zhu Y,et al.Preparation and corrosion assessment of electrodeposited Ni-SiC composite thin films[J].Ceramics International,2014,40(2):3341-3346.
- [9] 周月波,张海军.Ni-Al2O3纳米复合镀层的氧化性能研究[J].材料热处理学报,2008,29(2):154-157.ZHOU Yue-bo,ZHANG Hai-jun.Oxidation resistance of electrodeposited Ni-Al2O3 nanocomposite coating[J].Transactions of Materials and Heat Treatment,2008,29(2):154-157.
- [10] 黄柱,刘美霞,李天白,等.电沉积Ni-W-WC复合镀层摩擦磨损性能[J].有色金属科学与工程,2016,7(3):66-70.HUANG Zhu,LIU Mei-xia,LI Tian-bai,et al.Study on friction wear properties of Ni-W-WC composite coatings electrodeposition[J].Nonferrous Metals Science and Engineering,2016,7(3):66-70.
- [11] 耿浩,李金华,刘宣勇.石墨烯在表面工程领域的研究进展[J].中国表面工程,2015,28(1):4-14.GENG Hao,LI Jin-hua,LIU Xuan-yong.Research progress on graphene in surface engineering[J].China Surface Engineering,2015,28(1):4-14
- [12] Berry V.Impermeability of graphene and its applications[J].Carbon,2013,62(10):1-10.
- [13] Geim A K,Novoselov K S.The rise of graphene[J].Nature Materials,2007,6(3):183-191.
- [14] Berman D,Erdemir A,Sumant A V.Graphene:a new emerging lubricant[J].Materials Today,2014,17(1):31-42.
- [15] Shen X J,Pei X Q,Fu S Y,et al.Significantly modified tribological performance of epoxy nanocomposites at very low graphene oxide content[J].Polymer,2013,54(3):1234-1242.
- [16] 胡增荣,童国权,张超,等.激光烧结石墨烯钛纳米复合材料及其耐腐蚀性能[J].中国表面工程,2015,28(6):127-132.HU Zeng-rong,TONG Guo-quan,ZHANG Chao,et al.Corrosion behavior of laser sintered graphene reinforced titanium matrix nanocomposites[J].China Surface Engineering,2015,28(6):127-132.
- [17] Zhu Y,Murali S,Cai W,et al.Graphene and graphene oxide:synthesis,properties,and applications.[J].Advanced Materials,2010,22(35):3906-3924.
- [18] Yu Z,Di H,Ma Y,et al.Fabrication of graphene oxide-alumina hybrids to reinforce the anti-corrosion performance of composite epoxy coatings[J].Applied Surface Science,2015,351(1):986-996.
- [19] Pourhashem S,Vaezi M R,Rashidi A.Investigating the effect of SiO2-graphene oxide hybrid as inorganic nanofiller on corrosion protection properties of epoxy coatings[J].Surface and Coatings Technology,2017,311(15):282-294.
- [20] 王利,吴玉程,舒霞,等.低碳钢上Ni-W-Al2O3纳米复合电镀层的耐腐蚀性能研究[J].材料保护,2008,41(1):17-19.WANG Li,WU Yu-cheng,SHU Xia,et al.Corrosion resistance of Ni-W-Al2O3 nanocomposite coatings on low carbon steel[J].Materials Protection,2008,41(1):17-19.
- [21] 张玉碧,李照美,李云东,等.脉冲电镀中脉冲参数对镍镀层显微硬度的影响[J].电镀与涂饰,2005,24(2):1-3.ZHANG Yu-bi,LI Zhao-mei,LI Yun-dong,et al.Influences of pulse plating parameters on micro-hardness of nickel deposits[J].Electroplating and Finishing,2005,24(2):1-3.
- [22] 吴燕明,赵坚,陈小明,等.超音速喷涂纳米WC复合涂层与电镀铬层的组织及性能[J].材料热处理学报,2015,36(s1):171-176.WU Yan-ming,ZHAO Jian,CHEN Xiao-ming,et al.Microstructure and properties of high velocity sprayed nano WC composite coatings and chromium platings[J].Transactions of Materials and Heat Treatment,2015,36(s1):171-176.
- [23] 李晓闲,刘美霞,张雪辉,等.热处理对Ni-W-GO复合镀层组织及性能的影响[J].有色金属科学与工程,2017,8(5):115-120.LI Xiao-xian,LIU Mei-xia,ZHANG Xue-hui,et al.Effects of heat treatment on microstructure and properties of Ni-W-GO composite coatings[J].Nonferrous Metals Science and Engineering,2017,8(5):115-120.
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