核压力容器用SA508Gr.3钢的研究进展Research progress of SA508Gr.3 steel for nuclear pressure vessels
李林泽,代鑫,张源,周琳君,陈连生,田亚强
摘要(Abstract):
核反应堆压力容器是核电站重要组件且具有在全寿命周期内不可更换的特殊性。第二代核压力容器用钢在其焊缝中发现了再热裂纹,已不能够满足使用需求。因此,在此基础上通过添加Mn元素,减少Mo和Cr元素改进设计了SA508Gr.3钢,它具有高强度、高韧性和低辐照脆化敏感性等特点,目前广泛应用于核电压力容器、蒸发器和稳压器等核心构件。本文总结了SA508Gr.3钢的研究进展,重点介绍了合金元素、热处理工艺对其显微组织和力学性能的影响,并详细介绍了SA508Gr.3钢的抗辐照性能。根据核压力容器的服役环境,详细分析了热时效对SA508Gr.3钢显微组织及力学性能的影响机理。随后,总结了显微组织演化对其疲劳性能、疲劳裂纹萌生及疲劳裂纹扩展的影响机制。最后,展望了核压力容器的发展方向和需要进一步研究的内容,为提高SA508Gr.3钢的综合性能和研发下一代核电用钢提供参考。
关键词(KeyWords): 核压力容器;SA508Gr.3钢;热处理工艺;热时效;辐照;疲劳
基金项目(Foundation): 河北省自然科学基金(E2022209049);; 唐山市科技计划项目(22130206G);; 河北省高等学校科学研究项目(QN2023086);; 冶金与能源学院青年教师发展基金(YJY20244438)
作者(Author): 李林泽,代鑫,张源,周琳君,陈连生,田亚强
DOI: 10.13289/j.issn.1009-6264.2023-0550
参考文献(References):
- [1] 谢常胜.核用SA508Gr.3钢大锻件调质处理工艺、组织与性能研究[D].北京:北京科技大学,2020.XIE Chang-sheng.Study on heat treatment,microstructure and properties of SA508Gr.3 steel heavy forging for nuclear power plant[D].Beijing:University of Science and Technology Beijing,2020.
- [2] ASTM A508/A508M-18.Standard specification for quenched and tempered vacuum-treated carbon and alloy steel forgings for pressure vessels[S].United States:ASTM International,2018.
- [3] Im Y R,Lee B J,Yong J O,et al.Effect of microstructure on the cleavage fracture strength of low carbon Mn-Ni-Mo bainitic steels[J].Journal of Nuclear Materials,2004,324(1):33-40.
- [4] 胡本芙,卜勇,吴承建,等.N/Al比值对A508-3钢的组织和性能的影响[J].钢铁,1999(1):41-45.HU Ben-fu,PU Yong,WU Cheng-jian,et al.Effect of N/Al ratio on microstructure and properties of A508-3 steel for nuclear reactor pressure vessel[J].Iron and Steel,1999(1):41-45.
- [5] 王伟,隋大山,张佩佩,等.SA508-3钢保温过程奥氏体晶粒长大规律研究[J].热加工工艺,2013,42(16):31-34.WANG Wei,SUI Da-shan,ZHANG Pei-pei,et al.Austenite grain growth of SA508-3 steel in heating process[J].Hot Working Technology,2013,42(16):31-34.
- [6] 郭桢,刘建生,李景丹,等.核电SA508-3钢奥氏体晶粒长大规律的研究[J].大型铸锻件,2017(3):33-37.GUO Zhen,LIU Jian-sheng,LI Jing-dan,et al.Research on austenite grain growth behavior of nuclear power SA508-3 steel[J].Heavy Casting and Forging,2017(3):33-37.
- [7] 黄军波,何毅,赵美兰.淬火冷速对大型核电压力容器用钢显微组织和力学性能的影响[J].材料热处理学报,2020,41(4):158-164.HUANG Jun-bo,HE Yi,ZHAO Mei-lan.Effect of quenching cooling rate on microstructure and mechanical properties of heavy nuclear power pressure vessel steel[J].Transactions of Materials and Heat Treatment,2020,41(4):158-164.
- [8] 迟露鑫,麻永林,邢淑清,等.核电SA508-3钢在不同冷速下的显微组织[J].内蒙古科技大学学报,2010,29(2):127-131.CHI Lu-xin,MA Yong-lin,XING Shu-qing,et al.Microstructure of SA508-3 steel for nuclear power under different cooling rates[J].Journal of Inner Mongolia University of Science and Technology,2010,29(2):127-131.
- [9] 王天睿,张玉妥,王培.冷却速度对SA508-3钢显微组织与力学性能的影响[J].沈阳理工大学学报,2017,36(5):44-48.WANG Tian-rui,ZHANG Yu-tuo,WANG Pei.Effect of cooling rate on the microstructure and mechanical properties of SA508-3 steel[J].Journal of Shenyang Ligong University,2017,36(5):44-48.
- [10] 方才顺,王小彬,何西扣,等.淬火冷却速度和回火参数对核压力容器SA508-3钢强韧性的影响[J].金属热处理,2015,40(12):117-122.FANG Cai-shun,WANG Xiao-bin,HE Xi-kou,et al.Effects of quenching cooling rate and tempering parameters on strength and toughness of SA508-3 steel for nuclear pressure vessels[J].Heat Treatment of Metals,2015,40(12):117-122.
- [11] 马玉霞,党淑娥,秦尚武,等.SA508-3钢粗大非平衡组织重新加热奥氏体晶核形成与长大行为[J].金属热处理,2018,43(10):40-44.MA Yu-xia,DANG Shu-e,QIN Shang-wu,et al.Formation and growth behavior of austenite nuclei in coarse and non-equilibrium structure of SA508-3 steel during reheating[J].Heat Treatment of Metals,2018,43(10):40-44.
- [12] 董定乾,崔振山,陈飞.核电用SA508-3钢的奥氏体晶粒生长过程模拟[J].上海交通大学学报,2015,49(10):1504-1509.DONG Ding-qian,CUI Zhen-shan,CHEN Fei.Modeling of austenite grain growth of nuclear pressure vessel SA508-3 steel[J].Journal of Shanghai Jiao Tong University,2015,49(10):1504-1509.
- [13] 蒋中华,杜军毅,王培,等.M-A岛高温回火转变产物对核电SA508-3钢冲击韧性影响机制[J].金属学报,2021,57(7):891-902.JIANG Zhong-hua,DU Jun-yi,WANG Pei,et al.Mechanism of improving the impact toughness of SA508-3 steel used for nuclear power by pre-transformation of M-A islands[J].Acta Metallurgica Sinica,2021,57(7):891-902.
- [14] 王明敏,韩利战,顾剑锋.A508-3钢回火过程的组织演变及动力学分析[J].热处理,2013,28(6):19-24.WANG Ming-min,HAN Li-zhan,GU Jian-feng.Microstructure evolution of A508-3 steel during tempering and kinetic analysis[J].Heat Treatment,2013,28(6):19-24.
- [15] 盛钟琦,肖洪,彭峰.A508-3钢回火时显微组织的变化[J].核动力工程,1990(4):24-28.SHENG Zhong-qi,XIAO Hong,PENG Feng.The microstructural change of A508-3 steel during tempering[J].Nuclear Power Engineering,1990(4):24-28.
- [16] Jiang Z H,Li Y H,Yang Z D,et al.The tempering behavior of martensite/austenite islands on the mechanical properties of a low alloy Mn-Ni-Mo steel with granular bainite[J].Materials Today Communications,2021,26(12):102166.
- [17] 姜葳.质子辐照A508-3钢微结构演变规律[J].科技创新导报,2012,21:156.JIANG Wei.Evolution of microstructure of A508-3 steel by proton irradiation[J].Science and Technology Innovation Herald,2012,21:156.
- [18] 万强茂,束国刚,王荣山,等.A508-3钢质子辐照条件下微结构演变研究[J].金属学报,2012,48(8):929-934.WAN Qiang-mao,SHU Guo-gang,WANG Rong-shan,et al.Study on the microstructure evolution of A508-3 steel under proton irradiation[J].Acta Metallurgica Sinica,2012,48(8):929-934.
- [19] 林赟,宁广胜,张长义,等.国产A508-3钢辐照性能[J].原子能科学技术,2016,50(2):204-207.LIN Yun,NING Guang-sheng,ZHANG Chang-yi,et al.Mechanical property of China A508-3 steel after neutron irradiation[J].Atomic Energy Science and Technology,2016,50(2):204-207.
- [20] 丁兆楠,张宪龙,陈宇光,等.高能重离子辐照下国产RPV钢A508-3的硬化行为[J].装备环境工程,2022,19(1):39-44.DING Zhao-nan,ZHANG Xian-long,CHEN Yu-guang,et al.Hardening behavior of China RPV steel A508-3 under irradiation with high energy heavy ions[J].Equipment Environmental Engineering,2022,19(1):39-44.
- [21] 牛孟珂,韩旭孝,杨义涛,等.反应堆压力容器钢A508-3辐照硬化的剂量率效应研究[J].原子核物理评论,2021,38(4):438-443.NIU Meng-ke,HAN Xu-xiao,YANG Yi-tao,et al.Effect of the dose rate on irradiation hardening of reactor pressure vessel steel A508-3[J].Nuclear Physics Review,2021,38(4):438-443.
- [22] 张宪龙,吕康源,丁兆楠,等.小冲杆试验测定重离子辐照A508-3钢的硬化和脆化[J].装备环境工程,2022,19(1):45-49.ZHANG Xian-long,Lü Kang-yuan,DING Zhao-nan,et al.Determination of hardening and embrittlement of heavy-ion irradiated A508-3 steel by small punch test[J].Equipment Environmental Engineering,2022,19(1):45-49.
- [23] Liu X B,Wang R S,Jiang J,et al.Slow positron beam and nanoindentation study of irradiation-related defects in reactor vessel steels[J].Journal of Nuclear Materials,2014,451(1/3):249-254.
- [24] Wan Q M,Shu G G,Wang R S,et al.Characterization of proton irradiation-induced defect in the A508-3 steel by slow positron beam[J].Nuclear Inst and Methods in Physics Research B,2012,287:148-152.
- [25] Lin Y,Yang W,Tong Z F,et al.Charpy impact test on A508-3 steel after neutron irradiation[J].Engineering Failure Analysis,2017,82:733-740.
- [26] Zhou Z Y,Tong Z F,Qian G A,et al.Irradiation effect on impact fracture behavior of A508-3 steel in ductile-to-brittle transition range[J].Engineering Failure Analysis,2019,97:836-843.
- [27] 林虎,钟巍华,佟振峰,等.国产反应堆压力容器的辐照脆化行为及预测[J].原子能科学技术,2021,55(7):1170-1176.LIN Hu,ZHONG Wei-hua,TONG Zhen-feng,et al.Irradiation embrittlement behavior and prediction of domestic reactor pressure vessel[J].Atomic Energy Science and Technology,2021,55(7):1170-1176.
- [28] Li X H,Lei J,Shu G G,et al.A study on the microstructure and mechanical property of proton irradiated A508-3 steel[J].Nuclear Instruments and Methods in Physics Research B,2015,350:14-19.
- [29] Liu Y P,Nie J F,Lin P D,et al.Irradiation tensile property and fracture toughness evaluation study of A508-3 steel based on multi-scale approach[J].Annals of Nuclear Energy,2020,138:107157.
- [30] Ding Z N,Zhang C H,Zhang X L,et al.Post-irradiation annealing behavior of irradiation hardening of China low-Cu RPV steel[J].Nuclear Materials and Energy,2020,22:100727.
- [31] Lei J,Ding H,Shu G G,et al.Study on the mechanical properties evolution of A508-3 steel under proton irradiation[J].Nuclear Instruments and Methods in Physics Research Section B,2014,338:13-18.
- [32] Rodolfo K,Horacio T,Ana M F.Effect of lead factors on the embrittlement of RPV SA-508 cl 3 steel[J].Journal of Nuclear Materials,2013,434(1/3):411-416.
- [33] Marini B,Averty X,Wident P,et al.Effect of the bainitic and martensitic microstructures on the hardening and embrittlement under neutron irradiation of a reactor pressure vessel steel[J].Journal of Nuclear Materials,2015,465:20-27.
- [34] Druce S G,Gage G,Jordan G.Effect of ageing on properties of pressure vessel steels[J].Acta Metallurgica,1986,34(4):641-652.
- [35] Juichi F,Masayuk A,Masaaki K,et al.Effect of thermal aging on fracture toughness of RPV steel[J].Nuclear Engineering and Design,1993,144(3):423-429.
- [36] Wang W,Liu X J,Xu G,et al.Effect of thermal aging on microstructure and mechanical properties of China low-activation martensitic steel at 550 ℃[J].Nuclear Engineering and Technology,2016,48(2):518-524.
- [37] Vatter I A,Hippsley C A,Druce S G.Review of thermal ageing data and its application to operating reactor pressure vessels[J].International Journal of Pressure Vessels and Piping,1993,54(1/2):31-48.
- [38] Xing R S,Chen X,Yu D J.Evolution of impact properties of 16MND5 forgings for nuclear reactor pressure vessel during thermal aging at 500 ℃[J].Key Engineering Materials,2019,795:54-59.
- [39] Goritskii V M,Shneiderov G R,Shur A D,et al.Structural mechanism of the development of thermal embrittlement in steels with a temper-bainite structure[J].Metal Science and Heat Treatment,1992,34(1):3-9.
- [40] 邢睿思,陈旭,谢国福,等.热老化对于核电压力容器用钢16MND5冲击行为的影响[J].核动力工程,2018,39(2):104-108.XING Rui-si,CHEN Xu,XIE Guo-fu,et al.Effect of thermal aging on impact properties in 16MND5 forgings for nuclear reactor pressure vessel[J].Nuclear Power Engineering,2018,39(2):104-108.
- [41] Pareige P,Russell K F,Stoller R E,et al.Influence of long-term thermal aging on the microstructural evolution of nuclear reactor pressure vessel materials:An atom probe study[J].Journal of Nuclear Materials,1997,250(2):176-183.
- [42] Gunawardane H P,Hall J B,Rosinski S T,et al.Mechanical property changes in reactor vessel materials thermally aged for 209000 h at 260 ℃[J].Journal of ASTM International,2007,3(2):1-9.
- [43] 代鑫.核压力容器用大锻件SA508-Ⅳ钢疲劳性能的研究[D].北京:北京科技大学,2021.DAI Xin.A study on fatigue properties of heavy forging SA508-IV steel used for nuclear reactor pressure vessels[D].Beijing:University of Science and Technology Beijing,2021.
- [44] 任彬.核电用钢的多轴疲劳性能及预腐蚀疲劳性能研究[D].天津:天津大学,2018.REN Bin.A study on the multiaxial fatigue and pre-corroded fatigue behavior of nuclear power steels[D].Tianjin:Tianjin University,2018.
- [45] Dai X,Peng T,Chen Y F,et al.The correlation between martensite-austenite islands evolution and fatigue behavior of SA508-IV steel[J].International Journal of Fatigue,2020,139:105776.
- [46] Dai X,Chen Y,Wang P,et al.Mechanical and fatigue properties of SA508-IV steel used for nuclear reactor pressure vessels[J].Journal of Iron and Steel Research International,2022,29(8):1312-1321.
- [47] Souguir S,Brochard L,Sab K.Stress concentration and instabilities in the atomistic process of brittle failure initiation[J].International Journal of Fracture,2020,224(2):235-249.
- [48] Santofimia M J,Petrov R H,Zhao L,et al.Microstructural analysis of martensite constituents in quenching and partitioning steels[J].Materials Characterization,2014,92:91-95.
- [49] 武焕春.核电主管道不锈钢的腐蚀疲劳行为研究[D].北京:北京科技大学,2016.WU Huan-chun.Study on corrosion fatigue behaviors of primary coolant pipes on nuclear power plants[D].Beijing:University of Science and Technology Beijing,2016.
- [50] 田俊,唐妍婕,张丽屏,等.国产508-3钢不同温度下非比例多轴循环变形行为研究[J].核动力工程,2021,42(S2):89-92.TIAN Jun,TANG Yan-jie,ZHANG Li-ping,et al.Study of non-proportionally multiaxial cyclic deformation behavior of domestic 508-3 steel at different temperatures[J].Nuclear Power Engineering,2021,42(S2):89-92.
- [51] 刘哲,佟振峰,梁政强.国产A508-3钢的低周疲劳性能研究[J].原子能科学技术,2014,48(1):127-133.LIU Zhe,TONG Zhen-feng,LIANG Zheng-qiang.Investigation on low-cycle property of domestic A508-3 steel[J].Atomic Energy Science and Technology,2014,48(1):127-133.
- [52] 钟巍华,佟振峰,王成龙,等.国产A508-3钢在模拟AP1000一回路水环境下的疲劳性能研究[J].原子能科学技术,2020,54(4):702-708.ZHONG Wei-hua,TONG Zhen-feng,WANG Cheng-long,et al.Fatigue behavior of domestic A508-3 steel under simulated AP1000 primary coolant environment[J].Atomic Energy Science and Technology,2020,54(4):702-708.
- [53] 陆斌,丁亚平.国产低合金钢腐蚀疲劳和辐照脆化行为研究[J].腐蚀与防护,2001(11):463-467.LU Bin,DING Ya-ping.Corrosion fatigue and radiation brittlement behaviours of low alloy steel 508-3 produced in China[J].Corrosion and Protection,2001(11):463-467.
- [54] Bulloch J H.Influence of mean stress and frequency on the fatigue crack growth behaviour of A508cl III steel in a low temperature pressurised water reactor environment[J].International Journal of Pressure Vessels and Piping,1992,49(2):139-185.
- [55] Wu X,Katada Y.Cyclic cracking behavior of low-alloy pressure vessel steel in simulated BWR water[J].Journal of Nuclear Materials,2004,328(2):139-185.
- [56] Lu C Y,He Y M,Yang J G,et al.An investigation of phase transition on the microstructural characteristic and creep behavior for the SA508Gr.3 steel used for nuclear reactor pressure vessels[J].Materials Science and Engineering A,2018,711:659-669.
- [57] Srakra A,Sunil S,Kumawat B,et al.High temperature creep behavior of a low alloy Mn-Mo-Ni reactor pressure vessel steel[J].Journal of Nuclear Materials,2021,557:153293.
- [58] Gao Z L,Lu C Y,He Y M,et al.Influence of phase transformation on the creep deformation mechanism of SA508Gr.3 steel for nuclear reactor pressure vessels[J].Journal of Nuclear Materials,2019,519:292-301.
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